2D Layered SiP as Anisotropic Nonlinear Optical Material

Huseyin Sar; Jie Gao; Xiaodong Yang

doi:10.1038/s41598-021-85938-4

2D Layered SiP as Anisotropic Nonlinear Optical Material

Huseyin Sar
, Jie Gao
, Xiaodong Yang

Mechanical and Aerospace Engineering

Research output: Contribution to journal › Article › peer-review

Abstract

Two-dimensional (2D) material of silicon phosphide (SiP) has recently been shown as a promising optical material with large band gap, fast photoresponse and strong anisotropy. However, the nonlinear optical properties of 2D SiP have not been investigated yet. Here, the thickness-dependent in-plane anisotropic third-harmonic generation (THG) from the mechanically exfoliated 2D layered SiP flakes is reported. The crystal orientation of the SiP flake is determined by the angle-resolved polarized Raman spectroscopy. The angular dependence of the THG emission with respect to the incident linear polarization is found to be strongly anisotropic with the two-fold polarization dependence pattern. Furthermore, the effect of the SiP flake thickness on the THG power is analyzed.

Original language	American English
Article number	6372
Journal	Scientific Reports
Volume	11
Issue number	1
DOIs	https://doi.org/10.1038/s41598-021-85938-4
State	Published - Dec 1 2021

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Mechanical Engineering

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title = "2D Layered SiP as Anisotropic Nonlinear Optical Material",

abstract = " Two-dimensional (2D) material of silicon phosphide (SiP) has recently been shown as a promising optical material with large band gap, fast photoresponse and strong anisotropy. However, the nonlinear optical properties of 2D SiP have not been investigated yet. Here, the thickness-dependent in-plane anisotropic third-harmonic generation (THG) from the mechanically exfoliated 2D layered SiP flakes is reported. The crystal orientation of the SiP flake is determined by the angle-resolved polarized Raman spectroscopy. The angular dependence of the THG emission with respect to the incident linear polarization is found to be strongly anisotropic with the two-fold polarization dependence pattern. Furthermore, the effect of the SiP flake thickness on the THG power is analyzed.",

author = "Huseyin Sar and Jie Gao and Xiaodong Yang",

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year = "2021",

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doi = "10.1038/s41598-021-85938-4",

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T1 - 2D Layered SiP as Anisotropic Nonlinear Optical Material

AU - Sar, Huseyin

AU - Gao, Jie

AU - Yang, Xiaodong

PY - 2021/12/1

Y1 - 2021/12/1

N2 - Two-dimensional (2D) material of silicon phosphide (SiP) has recently been shown as a promising optical material with large band gap, fast photoresponse and strong anisotropy. However, the nonlinear optical properties of 2D SiP have not been investigated yet. Here, the thickness-dependent in-plane anisotropic third-harmonic generation (THG) from the mechanically exfoliated 2D layered SiP flakes is reported. The crystal orientation of the SiP flake is determined by the angle-resolved polarized Raman spectroscopy. The angular dependence of the THG emission with respect to the incident linear polarization is found to be strongly anisotropic with the two-fold polarization dependence pattern. Furthermore, the effect of the SiP flake thickness on the THG power is analyzed.

AB - Two-dimensional (2D) material of silicon phosphide (SiP) has recently been shown as a promising optical material with large band gap, fast photoresponse and strong anisotropy. However, the nonlinear optical properties of 2D SiP have not been investigated yet. Here, the thickness-dependent in-plane anisotropic third-harmonic generation (THG) from the mechanically exfoliated 2D layered SiP flakes is reported. The crystal orientation of the SiP flake is determined by the angle-resolved polarized Raman spectroscopy. The angular dependence of the THG emission with respect to the incident linear polarization is found to be strongly anisotropic with the two-fold polarization dependence pattern. Furthermore, the effect of the SiP flake thickness on the THG power is analyzed.

UR - https://scholarsmine.mst.edu/mec_aereng_facwork/4605

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DO - 10.1038/s41598-021-85938-4

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SN - 2045-2322

VL - 11

JO - Scientific Reports

JF - Scientific Reports

IS - 1

M1 - 6372

ER -

2D Layered SiP as Anisotropic Nonlinear Optical Material

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